Along with the three established first team players, goalkeepers Lars Hirschfeld and Shwan Jalal and defender Danny Foster have also left the club.
"I should like to thank the players and wish them well in the future," said Spurs chairman Daniel Levy.
"In particular we wish Darren well after no less than 12 years at the club.
"Gus and Christian have given the supporters much to cheer about during their stay, too. We wish them luck for the future."